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          我所二維有序介孔材料應用于微型超級電容器研究取得新進展

            近日,我所二維材料與能源器件創新特區研究組(DNL21T3)吳忠帥研究員團隊與上海交通大學麥亦勇教授團隊合作,發展了一種通用的界面自組裝策略,制備出一系列面內平行柱狀的有序介孔聚合物/石墨烯復合納米片,并將其應用于平面微型超級電容器,相關成果發表在《德國應用化學》(Angew. Chem. Int. Ed.)上。

            二維材料,如石墨烯,是一類具有重要應用前景的平面微型超級電容器電極材料。發展二維材料基復合介孔納米片,不僅可有效抑制片層的堆疊,增加比表面積,而且可大大緩沖電極的體積膨脹,提高電解液離子的擴散和電化學性能。但是,目前報道的都是關于面內垂直柱狀的介孔納米片,而面內平行柱狀的有序介孔納米片的可控制備仍面臨著很大挑戰。

            該研究團隊發展了一種普適的界面自組裝策略,制備出多種面內平行柱狀的有序介孔聚合物/石墨烯復合納米片,包括聚吡咯/石墨烯、聚苯胺/石墨烯、聚多巴胺/石墨烯,并將其應用于全固態平面微型超級電容器。這些納米片具有面內平行柱狀的有序介孔,大小為11-12nm,厚度為25-27nm,同時結合了高電化學活性的贗電容聚合物和高導電性的雙電層石墨烯的優勢。該工作獲得的微型超級電容器,表現出了高體積比容量和能量密度,同時還具有優異的機械柔性和串并聯集成性能。該工作為可控制備二維面內平行柱狀的有序介孔材料提供了新思路,為設計組裝高比能微型超級電容器提供了新策略。

            上述工作得到了國家自然科學基金、國家重點研發計劃等項目的資助。(文/圖 秦潔瓊、侯丹)

          版權所有 © 中國科學院大連化學物理研究所 本站內容如涉及知識產權問題請聯系我們 備案號:遼ICP備05000861號 遼公網安備21020402000367號
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